This Faculty Early Career Development (CAREER) award will support research that looks to derive a fundamental understanding of molecular interactions and toughening mechanisms in inorganic minerals for tailoring tough and durable structural materials. A key innovation is anticipate to lie in turning ubiquitous calcium carbonate into a monolithic binder as a potential alternative to cement and concrete, rather than a raw material thermally decomposed in traditional cement manufacturing. Towards this end, novel synthesis and strengthening pathways will be explored to address the fundamental challenges in constructing continuously structured inorganic monoliths and tackling the poor fracture toughness and low tensile strength of crystalline minerals. By redefining the synthesis process and improving the properties of materials and structures in a truly sustainable and cost-effective way, the anticipated project outcomes could ultimately shed light on multiple research areas and industrial sectors, including civil engineering, materials science, mechanical engineering, advanced manufacturing, and the utilization of abundant and renewable resources with long-term economic and environmental benefits. The research efforts will be integrated with educational activities, including the BRIGHT (Build Resilient, Innovative, and Green Homes on Terra), Science Playground, and SEED (Sustainability Exploration, Engagement, and Discovery) programs, to offer interactive, hands-on learning expe