Structural and Functional Properties of Enzymes Involved in Persulfide Degradation

NSF Award Search · 01002526DB NSF RESEARCH & RELATED ACTIVIT · $525,000 · view on nsf.gov ↗

Abstract

With support from the Chemistry of Life Processes Program in the Division of Chemistry, Professor Holly Ellis and her research team at East Carolina University will study the functional and structural attributes of a recently identified enzyme system that is metabolically relevant and involved in persulfide oxidation. The system consists of a mercaptopropionate dioxygenase (MDO) and a sulfurtransferase (ST), and it is involved in a novel pathway in persulfide oxidation. Interestingly, the MDO/ST enzymes have been identified in a wide range of bacteria, suggesting that it is critical to cellular function. Despite its ubiquity in bacteria, information about the mechanism of transformations catalyzed by the MDO/ST system is limited. The project focuses on filling this gap through the elucidation of the functional and structural properties of the enzymes. Graduate students engaged in this research are learning the biochemical and analytical skills needed to drive innovation in research and biotechnology. The project is also integrated with a pre-college program to train high school students in different biochemical techniques used to understand enzyme function. Oxidation and assimilation of persulfides in bacteria is often catalyzed by enzymes critical in maintaining potentially toxic persulfide levels and in supplying bacteria with alternative sulfur sources. The MDO thiol dioxygenases that catalyze the oxidation of low molecular weight (LMW) thiols were originally identif

Key facts

NSF award ID
2532276
Awardee
East Carolina University (NC)
SAM.gov UEI
HWPEKM8VFTJ9
PI
Holly R Ellis
Primary program
01002526DB NSF RESEARCH & RELATED ACTIVIT
All programs
Estimated total
$525,000
Funds obligated
$525,000
Transaction type
Standard Grant
Period
09/01/2025 → 08/31/2028